Control of quasi-phase-matching of high-harmonics in a spatially structured plasma

Wöstmann M, Splitthoff L, Zacharias H

Abstract

High-harmonic generation is widely used for providing extreme ultraviolet radiation in attosecond science. Such experiments include photoelectron spectroscopy, diffractive imaging, or the investigation of spin dynamics. Many applications are restricted by a low photon flux which originates from the low efficiency of the generation process. In this article an effective method based on the quasi-phase-matched generation of high harmonics in spatially structured, laser ablated plasma is demonstrated. Through a proper dimensioning of the plasma structure, the harmonic yield is optimized for a controllable range of harmonic orders. By using four coherent zones, the intensity of a single harmonic is increased to a maximal possible value of 16 compared to using a single zone. The Gouy phase shift of the fundamental field is identified as the primary effect responsible for constructive interference of the harmonic fields generated in the individual plasma jets of the plasma structure.