Motility-Induced Crystallization and Rotating Crystallites [Motilitätsinduzierte Kristallisation und rotierende Kristallite]

Holl, M. P.; Steinberg, A. B.; te Vrugt, M.; Thiele, U.

Research article (journal) | Peer reviewed

Abstract

Active soft matter frequently shows motility-induced phase separation, where self-propelled particles condensate into clusters with an inner liquidlike structure. Such activity may also result in motility-induced crystallization into clusters with an inner crystalline structure. We derive a higher-order active phase-field-crystal model and employ it to study the interplay of passive (i.e., thermodynamic) and active (i.e., motility-induced) condensation or evaporation and crystallization or melting. Stability and morphological phase diagrams indicate the various occurring phase coexistences and transitions, e.g., the destruction of passive clusters in the case of a density-independent effective velocity and the possible creation of active clusters in the case of a density-dependent effective velocity. Finally, simple and complex rotating crystallites are discussed, including states of time-periodic chirality.

Details about the publication

JournalPhysical Review Letters (Phys. Rev. Lett.)
Volume135
Article number158301
StatusPublished
Release year2025
Language in which the publication is writtenEnglish
DOI10.1103/m3dy-53yc
KeywordsPattern formation; Self-assembly; Collective dynamics; Living matter and active matter; Phase-field modeling; Theories of collective dynamics and active matter;

Authors from the University of Münster

Holl, Max Philipp
Professur für Theoretische Physik (Prof. Thiele)
Steinberg, Alina Barbara
Professur für Theoretische Physik (Prof. Thiele)
te Vrugt, Michael
Junior professorship for the theory of soft matter physics (Prof. Wittkowski)
Thiele, Uwe
Professur für Theoretische Physik (Prof. Thiele)
Center for Nonlinear Science
Center for Multiscale Theory and Computation (CMTC)
Center for Soft Nanoscience (SoN)

Promotionen, aus denen die Publikation resultiert

Pattern formation in Bose-Einstein condensates
Candidate: Steinberg, Alina Barbara | Supervisors: Thiele, Uwe; Gurevich, Svetlana; Maucher, Fabian
Period of time: 01/10/2020 - 30/09/2023
Doctoral examination procedure finished at: Doctoral examination procedure at University of Münster
Phase Field Crystal Models for active and passive soft matter
Candidate: Holl, Max Philipp | Supervisors: Thiele, Uwe; Archer, Andrew J:
Period of time: until 01/10/2022
Doctoral examination procedure finished at: Doctoral examination procedure at University of Münster